I'd definitely check with the hosting provider. They can check the SMTP logs and see if the mail is even making it to the server. 2 options at this point. Mail is being blocked from being sent through your ISP.. or mail is being rejected by your hosting provider for some reason.
Keep in mind ISP's will often block ports like 25 because they think if they allow it spammers will use their networks to send spam through. You might have to change ports. It MAY have worked in the past but the ISP could have changed policies or seen 'unusual' activity from your account and turned it on specifically for you thinking you were a spammer.